A novel natural drying (ND) strategy for low-cost and simple fabrication of graphene aerogels (GA) is highlighted. The as-formed NDGA exhibit ultralarge reversible compressibility (99%) and tunable Poisson's ratio behaviors (−0.30 < ν < 0.46), which suggests promising applications as soft actuators, soft robots, sensors, deformable electronic devices, drug release, thermal insulator, and protective materials.
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